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Joseph J, Holzmeier F, Bresteau D, Spezzani C, Ruchon T, Hergott JF, Tcherbakoff O, D'Oliveira P, Houver JC and Dowek D (2020), "Angle-resolved studies of XUV–IR two-photon ionization in the RABBITT scheme", Journal of Physics B: Atomic, Molecular and Optical Physics., aug, 2020. Vol. 53(18), pp. 184007. IOP Publishing.
BibTeX:
@article{Joseph2020,
  author = {J Joseph and F Holzmeier and D Bresteau and C Spezzani and T Ruchon and J F Hergott and O Tcherbakoff and P D'Oliveira and J C Houver and D Dowek},
  title = {Angle-resolved studies of XUV–IR two-photon ionization in the RABBITT scheme},
  journal = {Journal of Physics B: Atomic, Molecular and Optical Physics},
  publisher = {IOP Publishing},
  year = {2020},
  volume = {53},
  number = {18},
  pages = {184007},
  doi = {10.1088/1361-6455/ab9f0d}
}
Fanciulli M, Schusser J, Lee M-I, Youbi ZE, Heckmann O, Richter MC, Cacho C, Spezzani C, Bresteau D, Hergott J-F, D'Oliveira P, Tcherbakoff O, Ruchon T, Minár J and Hricovini K (2020), "Spin, time, and angle resolved photoemission spectroscopy on WTe2", Physical Review Research., mar, 2020. Vol. 2(1) American Physical Society (APS).
BibTeX:
@article{Fanciulli2020,
  author = {Mauro Fanciulli and Jakub Schusser and Min-I Lee and Zakariae El Youbi and Olivier Heckmann and Maria Christine Richter and Cephise Cacho and Carlo Spezzani and David Bresteau and Jean-François Hergott and Pascal D'Oliveira and Olivier Tcherbakoff and Thierry Ruchon and Jan Minár and Karol Hricovini},
  title = {Spin, time, and angle resolved photoemission spectroscopy on WTe2},
  journal = {Physical Review Research},
  publisher = {American Physical Society (APS)},
  year = {2020},
  volume = {2},
  number = {1},
  doi = {10.1103/physrevresearch.2.013261}
}
Buono WT, Santos A, Maia MR, Pereira LJ, Tasca DS, Dechoum K, Ruchon T and Khoury AZ (2020), "Chiral relations and radial-angular coupling in nonlinear interactions of optical vortices", Physical Review A., apr, 2020. Vol. 101(4) American Physical Society (APS).
BibTeX:
@article{Buono2020,
  author = {W. T. Buono and A. Santos and M. R. Maia and L. J. Pereira and D. S. Tasca and K. Dechoum and T. Ruchon and A. Z. Khoury},
  title = {Chiral relations and radial-angular coupling in nonlinear interactions of optical vortices},
  journal = {Physical Review A},
  publisher = {American Physical Society (APS)},
  year = {2020},
  volume = {101},
  number = {4},
  doi = {10.1103/physreva.101.043821}
}
Bourassin-Bouchet C, Barreau L, Gruson V, Hergott J-F, Quéré F, Salières P and Ruchon T (2020), "Quantifying Decoherence in Attosecond Metrology", Physical Review X., aug, 2020. Vol. 10(3) American Physical Society (APS).
BibTeX:
@article{BourassinBouchet2020,
  author = {C. Bourassin-Bouchet and L. Barreau and V. Gruson and J.-F. Hergott and F. Quéré and P. Salières and T. Ruchon},
  title = {Quantifying Decoherence in Attosecond Metrology},
  journal = {Physical Review X},
  publisher = {American Physical Society (APS)},
  year = {2020},
  volume = {10},
  number = {3},
  doi = {10.1103/physrevx.10.031048}
}
Chappuis C, Bresteau D, Auguste T, Gobert O and Ruchon T (2019), "High-order harmonic generation in an active grating", Physical Review A., mar, 2019. Vol. 99(3) American Physical Society (APS).
BibTeX:
@article{Chappuis2019,
  author = {C. Chappuis and D. Bresteau and T. Auguste and O. Gobert and T. Ruchon},
  title = {High-order harmonic generation in an active grating},
  journal = {Physical Review A},
  publisher = {American Physical Society (APS)},
  year = {2019},
  volume = {99},
  number = {3},
  doi = {10.1103/physreva.99.033806}
}
Gruson V, Weber SJ, Barreau L, Hergott J-F, Lepetit F, Auguste T, Carré B, Salières P and Ruchon T (2018), "Interferometric control of the ellipticity of a femtosecond extreme ultraviolet source", Journal of the Optical Society of America B., mar, 2018. Vol. 35(4), pp. A15. The Optical Society.
BibTeX:
@article{Gruson2018,
  author = {V. Gruson and S. J. Weber and L. Barreau and J.-F. Hergott and F. Lepetit and T. Auguste and B. Carré and P. Salières and T. Ruchon},
  title = {Interferometric control of the ellipticity of a femtosecond extreme ultraviolet source},
  journal = {Journal of the Optical Society of America B},
  publisher = {The Optical Society},
  year = {2018},
  volume = {35},
  number = {4},
  pages = {A15},
  doi = {10.1364/josab.35.000a15}
}
Gonzalez AI, Jargot G, Rigaud P, Lavenu L, Guichard F, Comby A, Auguste T, Sublemontier O, Bougeard M, Zaouter Y, Georges P, Hanna M and Ruchon T (2018), "Spatio-spectral structures in high harmonic generation driven by tightly focused high repetition rate lasers", Journal of the Optical Society of America B., feb, 2018. Vol. 35(4), pp. A6. The Optical Society.
BibTeX:
@article{Gonzalez2018,
  author = {Aura Inés Gonzalez and Gaëtan Jargot and Philippe Rigaud and Loïc Lavenu and Florent Guichard and Antoine Comby and Thierry Auguste and Olivier Sublemontier and Michel Bougeard and Yoann Zaouter and Patrick Georges and Marc Hanna and Thierry Ruchon},
  title = {Spatio-spectral structures in high harmonic generation driven by tightly focused high repetition rate lasers},
  journal = {Journal of the Optical Society of America B},
  publisher = {The Optical Society},
  year = {2018},
  volume = {35},
  number = {4},
  pages = {A6},
  doi = {10.1364/josab.35.0000a6}
}
Brauße F, Goldsztejn G, Amini K, Boll R, Bari S, Bomme C, Brouard M, Burt M, de Miranda BC, Düsterer S, Erk B, Géléoc M, Geneaux R, Gentleman AS, Guillemin R, Ismail I, Johnsson P, Journel L, Kierspel T, Köckert H, Küpper J, Lablanquie P, Lahl J, Lee JWL, Mackenzie SR, Maclot S, Manschwetus B, Mereshchenko AS, Mullins T, Olshin PK, Palaudoux J, Patchkovskii S, Penent F, Piancastelli MN, Rompotis D, Ruchon T, Rudenko A, Savelyev E, Schirmel N, Techert S, Travnikova O, Trippel S, Underwood JG, Vallance C, Wiese J, Simon M, Holland DMP, Marchenko T, Rouzée A and Rolles D (2018), "Time-resolved inner-shell photoelectron spectroscopy: From a bound molecule to an isolated atom", Physical Review A., apr, 2018. Vol. 97(4) American Physical Society (APS).
BibTeX:
@article{Brause2018,
  author = {Felix Brauße and Gildas Goldsztejn and Kasra Amini and Rebecca Boll and Sadia Bari and Cédric Bomme and Mark Brouard and Michael Burt and Barbara Cunha de Miranda and Stefan Düsterer and Benjamin Erk and Marie Géléoc and Romain Geneaux and Alexander S. Gentleman and Renaud Guillemin and Iyas Ismail and Per Johnsson and Loïc Journel and Thomas Kierspel and Hansjochen Köckert and Jochen Küpper and Pascal Lablanquie and Jan Lahl and Jason W. L. Lee and Stuart R. Mackenzie and Sylvain Maclot and Bastian Manschwetus and Andrey S. Mereshchenko and Terence Mullins and Pavel K. Olshin and Jérôme Palaudoux and Serguei Patchkovskii and Francis Penent and Maria Novella Piancastelli and Dimitrios Rompotis and Thierry Ruchon and Artem Rudenko and Evgeny Savelyev and Nora Schirmel and Simone Techert and Oksana Travnikova and Sebastian Trippel and Jonathan G. Underwood and Claire Vallance and Joss Wiese and Marc Simon and David M. P. Holland and Tatiana Marchenko and Arnaud Rouzée and Daniel Rolles},
  title = {Time-resolved inner-shell photoelectron spectroscopy: From a bound molecule to an isolated atom},
  journal = {Physical Review A},
  publisher = {American Physical Society (APS)},
  year = {2018},
  volume = {97},
  number = {4},
  doi = {10.1103/physreva.97.043429}
}
Allum F, Burt M, Amini K, Boll R, Köckert H, Olshin PK, Bari S, Bomme C, Brauße F, de Miranda BC, Düsterer S, Erk B, Géléoc M, Geneaux R, Gentleman AS, Goldsztejn G, Guillemin R, Holland DMP, Ismail I, Johnsson P, Journel L, Küpper J, Lahl J, Lee JWL, Maclot S, Mackenzie SR, Manschwetus B, Mereshchenko AS, Mason R, Palaudoux J, Piancastelli MN, Penent F, Rompotis D, Rouzée A, Ruchon T, Rudenko A, Savelyev E, Simon M, Schirmel N, Stapelfeldt H, Techert S, Travnikova O, Trippel S, Underwood JG, Vallance C, Wiese J, Ziaee F, Brouard M, Marchenko T and Rolles D (2018), "Coulomb explosion imaging of CH3I and CH2ClI photodissociation dynamics", The Journal of Chemical Physics., nov, 2018. Vol. 149(20), pp. 204313. AIP Publishing.
BibTeX:
@article{Allum2018,
  author = {Felix Allum and Michael Burt and Kasra Amini and Rebecca Boll and Hansjochen Köckert and Pavel K. Olshin and Sadia Bari and Cédric Bomme and Felix Brauße and Barbara Cunha de Miranda and Stefan Düsterer and Benjamin Erk and Marie Géléoc and Romain Geneaux and Alexander S. Gentleman and Gildas Goldsztejn and Renaud Guillemin and David M. P. Holland and Iyas Ismail and Per Johnsson and Loïc Journel and Jochen Küpper and Jan Lahl and Jason W. L. Lee and Sylvain Maclot and Stuart R. Mackenzie and Bastian Manschwetus and Andrey S. Mereshchenko and Robert Mason and Jérôme Palaudoux and Maria Novella Piancastelli and Francis Penent and Dimitrios Rompotis and Arnaud Rouzée and Thierry Ruchon and Artem Rudenko and Evgeny Savelyev and Marc Simon and Nora Schirmel and Henrik Stapelfeldt and Simone Techert and Oksana Travnikova and Sebastian Trippel and Jonathan G. Underwood and Claire Vallance and Joss Wiese and Farzaneh Ziaee and Mark Brouard and Tatiana Marchenko and Daniel Rolles},
  title = {Coulomb explosion imaging of CH3I and CH2ClI photodissociation dynamics},
  journal = {The Journal of Chemical Physics},
  publisher = {AIP Publishing},
  year = {2018},
  volume = {149},
  number = {20},
  pages = {204313},
  doi = {10.1063/1.5041381}
}
Géneaux R, Chappuis C, Auguste T, Beaulieu S, Gorman TT, Lepetit F, DiMauro LF and Ruchon T (2017), "Radial index of Laguerre-Gaussian modes in high-order-harmonic generation", Phys. Rev. A., May, 2017. Vol. 95, pp. 051801. American Physical Society.
BibTeX:
@article{GeneauxPRA2017,
  author = {Géneaux, Romain and Chappuis, Céline and Auguste, Thierry and Beaulieu, Samuel and Gorman, Timothy T. and Lepetit, Fabien and DiMauro, Louis F. and Ruchon, Thierry},
  title = {Radial index of Laguerre-Gaussian modes in high-order-harmonic generation},
  journal = {Phys. Rev. A},
  publisher = {American Physical Society},
  year = {2017},
  volume = {95},
  pages = {051801},
  url = {https://link.aps.org/doi/10.1103/PhysRevA.95.051801},
  doi = {10.1103/PhysRevA.95.051801}
}
Gauthier D, Ribič PR, Adhikary G, Camper A, Chappuis C, Cucini R, DiMauro LF, Dovillaire G, Frassetto F, Géneaux R, Miotti P, Poletto L, Ressel B, Spezzani C, Stupar M, Ruchon T and Ninno GD (2017), "Tunable orbital angular momentum in high-harmonic generation", Nature Communications., apr, 2017. Vol. 8, pp. 14971. Springer Nature.
BibTeX:
@article{Gauthier2017,
  author = {D. Gauthier and P. Rebernik Ribič and G. Adhikary and A. Camper and C. Chappuis and R. Cucini and L. F. DiMauro and G. Dovillaire and F. Frassetto and R. Géneaux and P. Miotti and L. Poletto and B. Ressel and C. Spezzani and M. Stupar and T. Ruchon and G. De Ninno},
  title = {Tunable orbital angular momentum in high-harmonic generation},
  journal = {Nature Communications},
  publisher = {Springer Nature},
  year = {2017},
  volume = {8},
  pages = {14971},
  doi = {10.1038/ncomms14971}
}
Camper A, Park H, Lai YH, Kageyama H, Li S, Talbert BK, Blaga CI, Agostini P, Ruchon T and DiMauro LF (2017), "Tunable mid-infrared source of light carrying orbital angular momentum in the femtosecond regime", Optics Letters., sep, 2017. Vol. 42(19), pp. 3769. The Optical Society.
BibTeX:
@article{Camper2017,
  author = {Antoine Camper and Hyunwook Park and Yu Hang Lai and Hiroyuki Kageyama and Sha Li and Bradford K. Talbert and Cosmin I. Blaga and Pierre Agostini and Thierry Ruchon and Louis F. DiMauro},
  title = {Tunable mid-infrared source of light carrying orbital angular momentum in the femtosecond regime},
  journal = {Optics Letters},
  publisher = {The Optical Society},
  year = {2017},
  volume = {42},
  number = {19},
  pages = {3769},
  doi = {10.1364/ol.42.003769}
}
Burt M, Boll R, Lee JWL, Amini K, Köckert H, Vallance C, Gentleman AS, Mackenzie SR, Bari S, Bomme C, Düsterer S, Erk B, Manschwetus B, Müller E, Rompotis D, Savelyev E, Schirmel N, Techert S, Treusch R, Küpper J, Trippel S, Wiese J, Stapelfeldt H, de Miranda BC, Guillemin R, Ismail I, Journel L, Marchenko T, Palaudoux J, Penent F, Piancastelli MN, Simon M, Travnikova O, Brausse F, Goldsztejn G, Rouzée A, Géléoc M, Geneaux R, Ruchon T, Underwood J, Holland DMP, Mereshchenko AS, Olshin PK, Johnsson P, Maclot S, Lahl J, Rudenko A, Ziaee F, Brouard M and Rolles D (2017), "Coulomb-explosion imaging of concurrent CH2BrI photodissociation dynamics", Physical Review A., oct, 2017. Vol. 96(4) American Physical Society (APS).
BibTeX:
@article{Burt2017,
  author = {Michael Burt and Rebecca Boll and Jason W. L. Lee and Kasra Amini and Hansjochen Köckert and Claire Vallance and Alexander S. Gentleman and Stuart R. Mackenzie and Sadia Bari and Cédric Bomme and Stefan Düsterer and Benjamin Erk and Bastian Manschwetus and Erland Müller and Dimitrios Rompotis and Evgeny Savelyev and Nora Schirmel and Simone Techert and Rolf Treusch and Jochen Küpper and Sebastian Trippel and Joss Wiese and Henrik Stapelfeldt and Barbara Cunha de Miranda and Renaud Guillemin and Iyas Ismail and Loïc Journel and Tatiana Marchenko and Jérôme Palaudoux and Francis Penent and Maria Novella Piancastelli and Marc Simon and Oksana Travnikova and Felix Brausse and Gildas Goldsztejn and Arnaud Rouzée and Marie Géléoc and Romain Geneaux and Thierry Ruchon and Jonathan Underwood and David M. P. Holland and Andrey S. Mereshchenko and Pavel K. Olshin and Per Johnsson and Sylvain Maclot and Jan Lahl and Artem Rudenko and Farzaneh Ziaee and Mark Brouard and Daniel Rolles},
  title = {Coulomb-explosion imaging of concurrent CH2BrI photodissociation dynamics},
  journal = {Physical Review A},
  publisher = {American Physical Society (APS)},
  year = {2017},
  volume = {96},
  number = {4},
  doi = {10.1103/physreva.96.043415}
}
Beaulieu S, Comby A, Clergerie A, Caillat J, Descamps D, Dudovich N, Fabre B, Géneaux R, Légaré F, Petit S, Pons B, Porat G, Ruchon T, Taïeb R, Blanchet V and Mairesse Y (2017), "Attosecond-resolved photoionization of chiral molecules", Science., dec, 2017. Vol. 358(6368), pp. 1288-1294. American Association for the Advancement of Science (AAAS).
BibTeX:
@article{Beaulieu2017,
  author = {S. Beaulieu and A. Comby and A. Clergerie and J. Caillat and D. Descamps and N. Dudovich and B. Fabre and R. Géneaux and F. Légaré and S. Petit and B. Pons and G. Porat and T. Ruchon and R. Taïeb and V. Blanchet and Y. Mairesse},
  title = {Attosecond-resolved photoionization of chiral molecules},
  journal = {Science},
  publisher = {American Association for the Advancement of Science (AAAS)},
  year = {2017},
  volume = {358},
  number = {6368},
  pages = {1288--1294},
  doi = {10.1126/science.aao5624}
}
Balogh E, Zhang C, Ruchon T, Hergott J-F, Quere F, Corkum P, Nam CH and Kim KT (2017), "Dynamic wavefront rotation in the attosecond lighthouse", Optica., Jan, 2017. Vol. 4(1), pp. 48. The Optical Society.
BibTeX:
@article{Balogh_2017,
  author = {Balogh, Emeric and Zhang, Chunmei and Ruchon, Thierry and Hergott, Jean-Francois and Quere, Fabien and Corkum, Paul and Nam, Chang Hee and Kim, Kyung Taec},
  title = {Dynamic wavefront rotation in the attosecond lighthouse},
  journal = {Optica},
  publisher = {The Optical Society},
  year = {2017},
  volume = {4},
  number = {1},
  pages = {48},
  url = {http://dx.doi.org/10.1364/OPTICA.4.000048},
  doi = {10.1364/optica.4.000048}
}
Veyrinas K, Gruson V, Weber SJ, Barreau L, Ruchon T, Hergott J-F, Houver J-C, Lucchese RR, Salières P and Dowek D (2016), "Molecular frame photoemission by a comb of elliptical high-order harmonics: a sensitive probe of both photodynamics and harmonic complete polarization state", Faraday Discussions. Vol. 194, pp. 161-183. Royal Society of Chemistry (RSC).
BibTeX:
@article{Veyrinas2016,
  author = {K. Veyrinas and V. Gruson and S. J. Weber and L. Barreau and T. Ruchon and J.-F. Hergott and J.-C. Houver and R. R. Lucchese and P. Salières and D. Dowek},
  title = {Molecular frame photoemission by a comb of elliptical high-order harmonics: a sensitive probe of both photodynamics and harmonic complete polarization state},
  journal = {Faraday Discussions},
  publisher = {Royal Society of Chemistry (RSC)},
  year = {2016},
  volume = {194},
  pages = {161--183},
  doi = {10.1039/c6fd00137h}
}
Gruson V, Barreau L, Jiménez-Galan Á, Risoud F, Caillat J, Maquet A, Carré B, Lepetit F, Hergott J-F, Ruchon T, Argenti L, Ta\ieb R, Mart\in F and Salières P (2016), "Attosecond dynamics through a Fano resonance: Monitoring the birth of a photoelectron", Science. Vol. 354(6313), pp. 734-738. American Association for the Advancement of Science.
Abstract: Theorists have long pondered the underpinnings of the Fano resonance, a spectral feature that resembles adjacent rightside-up and upside-down peaks. An especially well-studied instance of this feature appears in the electronic spectrum of helium as a transient state undergoes delayed ionization. Two studies have now traced the dynamics of this state in real time. Gruson et al. used photoelectron spectroscopy to extract the amplitude and phase of the electron wave packet after inducing its interference with reference wave packets tuned into resonance at variable delays. Kaldun et al. used extreme ultraviolet absorption spectroscopy to probe the transient state while variably forcing ionization with a strong near-infrared field.Science, this issue pp. 734 and 738The dynamics of quantum systems are encoded in the amplitude and phase of wave packets. However, the rapidity of electron dynamics on the attosecond scale has precluded the complete characterization of electron wave packets in the time domain. Using spectrally resolved electron interferometry, we were able to measure the amplitude and phase of a photoelectron wave packet created through a Fano autoionizing resonance in helium. In our setup, replicas obtained by two-photon transitions interfere with reference wave packets that are formed through smooth continua, allowing the full temporal reconstruction, purely from experimental data, of the resonant wave packet released in the continuum. In turn, this resolves the buildup of the autoionizing resonance on an attosecond time scale. Our results, in excellent agreement with ab initio time-dependent calculations, raise prospects for detailed investigations of ultrafast photoemission dynamics governed by electron correlation, as well as coherent control over structured electron wave packets.
BibTeX:
@article{Gruson_2016,
  author = {Gruson, V. and Barreau, L. and Jiménez-Galan, Á. and Risoud, F. and Caillat, J. and Maquet, A. and Carré, B. and Lepetit, F. and Hergott, J.-F. and Ruchon, T. and Argenti, L. and Ta\ieb, R. and Mart\in, F. and Salières, P.},
  title = {Attosecond dynamics through a Fano resonance: Monitoring the birth of a photoelectron},
  journal = {Science},
  publisher = {American Association for the Advancement of Science},
  year = {2016},
  volume = {354},
  number = {6313},
  pages = {734--738},
  url = {http://science.sciencemag.org/content/354/6313/734},
  doi = {10.1126/science.aah5188}
}
Géneaux R, Camper A, Auguste T, Gobert O, Caillat J, Taïeb R and Ruchon T (2016), "Synthesis and characterization of attosecond light vortices in the extreme ultraviolet", Nature Communications., Aug, 2016. Vol. 7, pp. 12583. Springer Nature.
BibTeX:
@article{GeneauxNcom2016,
  author = {Géneaux, R. and Camper, A. and Auguste, T. and Gobert, O. and Caillat, J. and Taïeb, R. and Ruchon, T.},
  title = {Synthesis and characterization of attosecond light vortices in the extreme ultraviolet},
  journal = {Nature Communications},
  publisher = {Springer Nature},
  year = {2016},
  volume = {7},
  pages = {12583},
  url = {http://dx.doi.org/10.1038/ncomms12583},
  doi = {10.1038/ncomms12583}
}
Beaulieu S, Ferré A, Géneaux R, Canonge R, Descamps D, Fabre B, Fedorov N, Légaré F, Petit S, Ruchon T, Blanchet V, Mairesse Y and Pons B (2016), "Universality of photoelectron circular dichroism in the photoionization of chiral molecules", New Journal of Physics. Vol. 18(10), pp. 102002.
Abstract: Photoionization of chiral molecules by circularly polarized radiation gives rise to a strong forward/backward asymmetry in the photoelectron angular distribution, referred to as photoelectron circular dichroism (PECD). Here we show that PECD is a universal effect that reveals the inherent chirality of the target in all ionization regimes: single photon, multiphoton, above-threshold and tunnel ionization. These different regimes provide complementary spectroscopic information at electronic and vibrational levels. The universality of the PECD can be understood in terms of a classical picture of the ionizing process, in which electron scattering on the chiral potential under the influence of a circularly polarized electric field results in a strong forward/backward asymmetry.
BibTeX:
@article{BeaulieuNJP2016,
  author = {S Beaulieu and A Ferré and R Géneaux and R Canonge and D Descamps and B Fabre and N Fedorov and F Légaré and S Petit and T Ruchon and V Blanchet and Y Mairesse and B Pons},
  title = {Universality of photoelectron circular dichroism in the photoionization of chiral molecules},
  journal = {New Journal of Physics},
  year = {2016},
  volume = {18},
  number = {10},
  pages = {102002},
  url = {http://stacks.iop.org/1367-2630/18/i=10/a=102002}
}
Beaulieu S, Comby A, Fabre B, Descamps D, Ferre A, Garcia G, Geneaux R, Legare F, Nahon L, Petit S, Ruchon T, Pons B, Blanchet V and Mairesse Y (2016), "Probing ultrafast dynamics of chiral molecules using time-resolved photoelectron circular dichroism", Faraday Discuss.. Vol. 194, pp. 325-348. The Royal Society of Chemistry.
Abstract: Measuring the ultrafast dynamics of chiral molecules in the gas phase has been a long standing and challenging quest of molecular physics. The main limitation to reach that goal has been the lack of highly sensitive chiroptical measurement. By enabling chiral discrimination with up to several 10% of sensitivity, photoelectron circular dichroism (PECD) offers a solution to this issue. However, tracking ultrafast processes requires measuring PECD with ultrashort light pulses. Here we compare the PECD obtained with different light sources, from the extreme ultraviolet to the mid-infrared range, leading to different ionization regimes: single-photon, resonance-enhanced multiphoton, above-threshold and tunnel ionization. We use single and multiphoton ionization to probe the ultrafast relaxation of fenchone molecules photoexcited in their first Rydberg states. We show that time-resolved PECD enables revealing dynamics much faster than the population decay of the Rydberg states, demonstrating the high sensitivity of this technique to vibronic relaxation.
BibTeX:
@article{BeaulieuFD2016,
  author = {Beaulieu, Samuel and Comby, Antoine and Fabre, Baptiste and Descamps, Dominique and Ferre, Amelie and Garcia, Gustavo and Geneaux, Romain and Legare, Francois and Nahon, Laurent and Petit, Stephane and Ruchon, Thierry and Pons, Bernard and Blanchet, Valerie and Mairesse, Yann},
  title = {Probing ultrafast dynamics of chiral molecules using time-resolved photoelectron circular dichroism},
  journal = {Faraday Discuss.},
  publisher = {The Royal Society of Chemistry},
  year = {2016},
  volume = {194},
  pages = {325-348},
  url = {http://dx.doi.org/10.1039/C6FD00113K},
  doi = {10.1039/C6FD00113K}
}
Auguste T, Gobert O, Ruchon T and Quéré F (2016), "Attosecond lighthouses in gases: A theoretical and numerical study", Phys. Rev. A., Mar, 2016. Vol. 93, pp. 033825. American Physical Society.
BibTeX:
@article{AugustePRA2016,
  author = {Auguste, T. and Gobert, O. and Ruchon, T. and Quéré, F.},
  title = {Attosecond lighthouses in gases: A theoretical and numerical study},
  journal = {Phys. Rev. A},
  publisher = {American Physical Society},
  year = {2016},
  volume = {93},
  pages = {033825},
  url = {http://link.aps.org/doi/10.1103/PhysRevA.93.033825},
  doi = {10.1103/PhysRevA.93.033825}
}
Weber SJ, Manschwetus B, Billon M, Böttcher M, Bougeard M, Breger P, Géléoc M, Gruson V, Huetz A, Lin N, Picard YJ, Ruchon T, Salières P and Carré B (2015), "Flexible attosecond beamline for high harmonic spectroscopy and XUV/near-IR pump probe experiments requiring long acquisition times", Review of Scientific Instruments. Vol. 86(3)
BibTeX:
@article{WeberRSI2015,
  author = {Weber, S. J. and Manschwetus, B. and Billon, M. and Böttcher, M. and Bougeard, M. and Breger, P. and Géléoc, M. and Gruson, V. and Huetz, A. and Lin, N. and Picard, Y. J. and Ruchon, T. and Salières, P. and Carré, B.},
  title = {Flexible attosecond beamline for high harmonic spectroscopy and XUV/near-IR pump probe experiments requiring long acquisition times},
  journal = {Review of Scientific Instruments},
  year = {2015},
  volume = {86},
  number = {3},
  url = {http://scitation.aip.org/content/aip/journal/rsi/86/3/10.1063/1.4914464},
  doi = {10.1063/1.4914464}
}
Manschwetus B, Lin N, Rothhardt J, Guichard R, Auguste T, Camper A, Breger P, Caillat J, Géléoc M, Ruchon T, Taïeb R, Carré B and Salières P (2015), "Self-Probing Spectroscopy of the SF6 Molecule: A Study of the Spectral Amplitude and Phase of the High Harmonic Emission", The Journal of Physical Chemistry A. Vol. 119(23), pp. 6111-6122.
BibTeX:
@article{ManschwetusJPC2015,
  author = {Bastian Manschwetus and Nan Lin and Jan Rothhardt and Roland Guichard and Thierry Auguste and Antoine Camper and Pierre Breger and Jérémie Caillat and Marie Géléoc and Thierry Ruchon and Richard Taïeb and Bertrand Carré and Pascal Salières},
  title = {Self-Probing Spectroscopy of the SF6 Molecule: A Study of the Spectral Amplitude and Phase of the High Harmonic Emission},
  journal = {The Journal of Physical Chemistry A},
  year = {2015},
  volume = {119},
  number = {23},
  pages = {6111-6122},
  note = {PMID: 25812633},
  url = {http://dx.doi.org/10.1021/acs.jpca.5b00446},
  doi = {10.1021/acs.jpca.5b00446}
}
Ferré A, Handschin C, Dumergue M, Burgy F, Comby A, Descamps D, Fabre B, Garcia GA, Géneaux R, Merceron L, Mével E, Nahon L, Petit S, Pons B, Staedter D, Weber S, Ruchon T, Blanchet V and Mairesse Y (2015), "A table-top ultrashort light source in the extreme ultraviolet for circular dichroism experiments", Nature Photonics., feb, 2015. Vol. 9, pp. 93-98.
BibTeX:
@article{FerreNPhoton2015,
  author = {A. Ferré and Handschin, C. and Dumergue, M. and Burgy, F. and Comby, A. and Descamps, D. and Fabre, B. and Garcia, G. A. and Géneaux, R. and Merceron, L. and Mével, E. and Nahon, L. and Petit, S. and Pons, B. and Staedter, D. and Weber, S. and Ruchon, T. and Blanchet, V. and Mairesse, Y.},
  title = {A table-top ultrashort light source in the extreme ultraviolet for circular dichroism experiments},
  journal = {Nature Photonics},
  year = {2015},
  volume = {9},
  pages = {93-98},
  doi = {10.1038/nphoton.2014.314}
}
Ferré A, Boguslavskiy AE, Dagan M, Blanchet V, Bruner BD, Burgy F, Camper A, Descamps D, Fabre B, Fedorov N, Gaudin J, Geoffroy G, Mikosch J, Patchkovskii S, Petit S, Ruchon T, Soifer H, Staedter D, Wilkinson I, Stolow A, Dudovich N and Mairesse Y (2015), "Multi-channel electronic and vibrational dynamics in polyatomic resonant high-order harmonic generation", Nature Communications., January, 2015. Vol. 6, pp. 5952.
BibTeX:
@article{FerreNC2015,
  author = {Ferré, A. and Boguslavskiy, A. E. and Dagan, M. and Blanchet, V. and Bruner, B. D. and Burgy, F. and Camper, A. and Descamps, D. and Fabre, B. and Fedorov, N. and Gaudin, J. and Geoffroy, G. and Mikosch, J. and Patchkovskii, S. and Petit, S. and Ruchon, T. and Soifer, H. and Staedter, D. and Wilkinson, I. and Stolow, A. and Dudovich, N. and Mairesse, Y.},
  title = {Multi-channel electronic and vibrational dynamics in polyatomic resonant high-order harmonic generation},
  journal = {Nature Communications},
  year = {2015},
  volume = {6},
  pages = {5952},
  doi = {10.1038/ncomms6952}
}
Camper A, Ferré A, Lin N, Skantzakis E, Staedter D, English E, Manschwetus B, Burgy F, Petit S, Descamps D, Auguste T, Gobert O, Carré B, Salières P, Mairesse Y and Ruchon T (2015), "Transverse Electromagnetic Mode Conversion for High-Harmonic Self-Probing Spectroscopy", Photonics. Vol. 2(1), pp. 184.
BibTeX:
@article{CamperPhotonics2015,
  author = {Camper, Antoine and Ferré, Amélie and Lin, Nan and Skantzakis, Emmanouil and Staedter, David and English, Elizabeth and Manschwetus, Bastian and Burgy, Frédéric and Petit, Stéphane and Descamps, Dominique and Auguste, Thierry and Gobert, Olivier and Carré, Bertrand and Salières, Pascal and Mairesse, Yann and Ruchon, Thierry},
  title = {Transverse Electromagnetic Mode Conversion for High-Harmonic Self-Probing Spectroscopy},
  journal = {Photonics},
  year = {2015},
  volume = {2},
  number = {1},
  pages = {184},
  url = {http://www.mdpi.com/2304-6732/2/1/184},
  doi = {10.3390/photonics2010184}
}
Camper A, Ferré A, Blanchet V, Burgy F, Descamps D, Petit S, Ruchon T and Mairesse Y (2015), "Combined high-harmonic interferometries for vectorial spectroscopy", Opt. Lett.., Nov, 2015. Vol. 40(22), pp. 5387-5390. OSA.
Abstract: We present a new method to characterize transverse vectorial light produced by high-harmonic generation (HHG). The incoherent sum of the two components of the electric field is measured using a bi-dimensional transient grating while one of the components is simultaneously characterized using two-source interferometry. The combination of these two interferometric setups enables the amplitude and phase measurement of the two vectorial components of the extreme ultraviolet radiation. We demonstrate the potential of this technique in the case of HHG in aligned nitrogen, revealing the vectorial properties of harmonics 9&x2013;17 of a Ti:sapphire laser.
BibTeX:
@article{CamperOL2015,
  author = {Antoine Camper and Amélie Ferré and Valérie Blanchet and Frédéric Burgy and Dominique Descamps and Stéphane Petit and Thierry Ruchon and Yann Mairesse},
  title = {Combined high-harmonic interferometries for vectorial spectroscopy},
  journal = {Opt. Lett.},
  publisher = {OSA},
  year = {2015},
  volume = {40},
  number = {22},
  pages = {5387--5390},
  url = {http://ol.osa.org/abstract.cfm?URI=ol-40-22-5387},
  doi = {10.1364/OL.40.005387}
}
Quéré F, Vincenti H, Borot A, Monchocé S, Hammond TJ, Kim KT, Wheeler JA, Zhang C, Ruchon T, Auguste T, Hergott JF, Villeneuve DM, Corkum PB and Lopez-Martens R (2014), "Applications of ultrafast wavefront rotation in highly nonlinear optics", Journal of Physics B: Atomic, Molecular and Optical Physics. Vol. 47(12), pp. 124004.
Abstract: This paper provides an overview of ultrafast wavefront rotation of femtosecond laser pulses and its various applications in highly nonlinear optics, focusing on processes that lead to the generation of high-order harmonics and attosecond pulses. In this context, wavefront rotation can be exploited in different ways, to obtain new light sources for time-resolved studies, called â??attosecond lighthousesâ??, to perform time-resolved measurements of nonlinear optical processes, using â??photonic streakingâ??, or to track changes in the carrierâ??envelope relative phase of femtosecond laser pulses. The basic principles are explained qualitatively from different points of view, the experimental evidence obtained so far is summarized, and the perspectives opened by these effects are discussed.
BibTeX:
@article{QuereJPB2014,
  author = {F Quéré and H Vincenti and A Borot and S Monchocé and T J Hammond and Kyung Taec Kim and J A Wheeler and Chunmei Zhang and T Ruchon and T Auguste and J F Hergott and D M Villeneuve and P B Corkum and R Lopez-Martens},
  title = {Applications of ultrafast wavefront rotation in highly nonlinear optics},
  journal = {Journal of Physics B: Atomic, Molecular and Optical Physics},
  year = {2014},
  volume = {47},
  number = {12},
  pages = {124004},
  url = {http://stacks.iop.org/0953-4075/47/i=12/a=124004}
}
Picard YJ, Manschwetus B, Géléoc M, Böettcher M, Casagrande EMS, Lin N, Ruchon T, Carré B, Hergott J-F, Lepetit F, Ta\ieb R, Maquet A and Huetz A (2014), "Attosecond evolution of energy- and angle-resolved photoemission spectra in two-color (XUV + IR) ionization of rare gases", Phys. Rev. A., Mar, 2014. Vol. 89, pp. 031401. American Physical Society.
BibTeX:
@article{PicardPRA2014,
  author = {Picard, Y. J. and Manschwetus, B. and Géléoc, M. and Böettcher, M. and Casagrande, E. M. Staicu and Lin, N. and Ruchon, T. and Carré, B. and Hergott, J.-F. and Lepetit, F. and Ta\ieb, R. and Maquet, A. and Huetz, A.},
  title = {Attosecond evolution of energy- and angle-resolved photoemission spectra in two-color (XUV + IR) ionization of rare gases},
  journal = {Phys. Rev. A},
  publisher = {American Physical Society},
  year = {2014},
  volume = {89},
  pages = {031401},
  url = {http://link.aps.org/doi/10.1103/PhysRevA.89.031401},
  doi = {10.1103/PhysRevA.89.031401}
}
Forget N, Joffre M and Ruchon T (2014), "Ultrashort Light Sources", In Laser. , pp. 73-91. WORLD SCIENTIFIC.
BibTeX:
@inbook{Forget2014,
  author = {Nicolas Forget and Manuel Joffre and Thierry Ruchon},
  title = {Ultrashort Light Sources},
  booktitle = {Laser},
  publisher = {WORLD SCIENTIFIC},
  year = {2014},
  pages = {73-91},
  url = {http://www.worldscientific.com/doi/abs/10.1142/9789814612418_0004},
  doi = {10.1142/9789814612418_0004}
}
Diveki Z, Bourassin-Bouchet C, de Rossi S, English E, Meltchakov E, Gobert O, Guénot D, Carré B, Salières P, Ruchon T and Delmotte F (2014), "Theoretical and experimental studies of broadband phase-controlled attosecond mirrors", Journal of Modern Optics. Vol. 61(2), pp. 122-131.
BibTeX:
@article{DivekiJMO2014,
  author = {Diveki, Z. and Bourassin-Bouchet, C. and de Rossi, S. and English, E. and Meltchakov, E. and Gobert, O. and Guénot, D. and Carré, B. and Salières, P. and Ruchon, T. and Delmotte, F.},
  title = {Theoretical and experimental studies of broadband phase-controlled attosecond mirrors},
  journal = {Journal of Modern Optics},
  year = {2014},
  volume = {61},
  number = {2},
  pages = {122-131},
  url = {http://dx.doi.org/10.1080/09500340.2013.869016},
  doi = {10.1080/09500340.2013.869016}
}
Camper A, Ruchon T, Gauthier D, Gobert O, Salières P, Carré B and Auguste T (2014), "High-harmonic phase spectroscopy using a binary diffractive optical element", Phys. Rev. A., Apr, 2014. Vol. 89, pp. 043843. American Physical Society.
BibTeX:
@article{CamperPRA2014,
  author = {Camper, A. and Ruchon, T. and Gauthier, D. and Gobert, O. and Salières, P. and Carré, B. and Auguste, T.},
  title = {High-harmonic phase spectroscopy using a binary diffractive optical element},
  journal = {Phys. Rev. A},
  publisher = {American Physical Society},
  year = {2014},
  volume = {89},
  pages = {043843},
  url = {http://link.aps.org/doi/10.1103/PhysRevA.89.043843},
  doi = {10.1103/PhysRevA.89.043843}
}
Kim KT, Zhang C, Ruchon T, Hergott J-F, Auguste T, Villeneuve DM, Corkum PB and Quéré F (2013), "Photonic streaking of attosecond pulse trains", Nature Photonics., August, 2013. Vol. 7, pp. 651-656.
BibTeX:
@article{KimNP2013,
  author = {Kim, K. T. and Zhang, C. and Ruchon, T. and Hergott, J.-F. and Auguste, T. and Villeneuve, D. M. and Corkum, P. B. and Quéré, F.},
  title = {Photonic streaking of attosecond pulse trains},
  journal = {Nature Photonics},
  year = {2013},
  volume = {7},
  pages = {651-656},
  doi = {10.1038/nphoton.2013.170}
}
Diveki Z, Guichard R, Caillat J, Camper A, Haessler S, Auguste T, Ruchon T, Carré B, Maquet A, Ta\ieb R and Salières P (2013), "Molecular orbital tomography from multi-channel harmonic emission in N2\", Chemical Physics. Vol. 414(0), pp. 121 - 129.
Abstract: High-order harmonic generation in aligned molecules can be used as an ultrafast probe of molecular structure and dynamics. By characterizing the emitted signal, one can retrieve information about electronic and nuclear dynamics at the attosecond timescale. In this paper, we discuss the theoretical and experimental aspects of molecular orbital tomography in N 2 and investigate the influence of multi-channel ionization on the orbital imaging. By analyzing the harmonicsâ?? spectral phase as a function of the driving laser intensity, we address two distinct cases, which in principle allow the orbital reconstruction. First, the contributions from two molecular orbitals could be disentangled in the real and imaginary parts of the measured dipole, allowing to reconstruct both orbitals. Second, by decreasing the driving laser intensity, the transition from a multi-channel to a single-channel ionization regime is shown. The latter approach paves the way towards the generalization of tomography to more complex systems.
BibTeX:
@article{DivekiCP2013,
  author = {Z. Diveki and R. Guichard and J. Caillat and A. Camper and S. Haessler and T. Auguste and T. Ruchon and B. Carré and A. Maquet and R. Ta\ieb and P. Salières},
  title = {Molecular orbital tomography from multi-channel harmonic emission in N2\},
  journal = {Chemical Physics},
  year = {2013},
  volume = {414},
  number = {0},
  pages = {121 - 129},
  url = {http://www.sciencedirect.com/science/article/pii/S0301010412001401},
  doi = {10.1016/j.chemphys.2012.03.021}
}
Diveki Z, Camper A, Haessler S, Auguste T, Ruchon T, Carré B, Salières P, Guichard R, Caillat J, Maquet A and Ta\ieb R (2012), "Spectrally resolved multi-channel contributions to the harmonic emission in N 2", New Journal of Physics. Vol. 14(2), pp. 023062.
Abstract: When generated in molecules, high-order harmonics can be emitted through different ionization channels. The coherent and ultrafast electron dynamics occurring in the ion during the generation process is directly imprinted in the harmonic signal, i.e. in its amplitude and spectral phase. In aligned N 2 molecules, we find evidence for a fast variation of this phase as a function of the harmonic order when varying the driving laser intensity. Basing our analysis on a three-step model, we find that this phase variation is a signature of transitions from a single- to a multi-channel regime. In particular, we show that significant nuclear dynamics may occur in the ionization channels on the attosecond timescale, affecting both the amplitude and the phase of the harmonic signal.
BibTeX:
@article{DivekiNJP2012,
  author = {Z Diveki and A Camper and S Haessler and T Auguste and T Ruchon and B Carré and P Salières and R Guichard and J Caillat and A Maquet and R Ta\ieb},
  title = {Spectrally resolved multi-channel contributions to the harmonic emission in N 2},
  journal = {New Journal of Physics},
  year = {2012},
  volume = {14},
  number = {2},
  pages = {023062},
  url = {http://stacks.iop.org/1367-2630/14/i=2/a=023062}
}
Billaud P, Géléoc M, Picard YJ, Veyrinas K, Hergott JF, Poullain SM, Breger P, Ruchon T, Roulliay M, Delmotte F, Lepetit F, Huetz A, Carré B and Dowek D (2012), "Molecular frame photoemission in dissociative ionization of H2 and D2 induced by high harmonic generation femtosecond XUV pulses", Journal of Physics B: Atomic, Molecular and Optical Physics. Vol. 45(19), pp. 194013.
Abstract: We report the first results of molecular frame photoelectron emission for dissociative photoionization (DPI) of H 2 and D 2 molecules induced by a spectrally filtered single high harmonic of a few femtosecond duration, using coincident electronââ?¬â??ion velocity vector correlation techniques. For the studied photon energies around 32Ã? eV, where the resonant excitation of the Q 1Ã? and Q 2 Ã? doubly excited states occurs, autoionization and nuclear dynamics are coupled on a few femtosecond timescale, giving rise to quantum interferences. Molecular frame photoelectron angular distributions (MFPADs), traced as a function of the kinetic energy release of the atomic fragments, provide the most sensitive observables for such complex dynamics. These results compare well with recent spectrally resolved experiments using synchrotron radiation which are also reported. As a novel XUV light source running at multi-kHz repetition rate and synchronized with laser pulses, high-order harmonic generation (HHG) opens new possibilities for extending these investigations to time-resolved studies at the femtosecond scale.
BibTeX:
@article{BillaudJPB2012,
  author = {P Billaud and M Géléoc and Y J Picard and K Veyrinas and J F Hergott and S Marggi Poullain and P Breger and T Ruchon and M Roulliay and F Delmotte and F Lepetit and A Huetz and B Carré and D Dowek},
  title = {Molecular frame photoemission in dissociative ionization of H2 and D2 induced by high harmonic generation femtosecond XUV pulses},
  journal = {Journal of Physics B: Atomic, Molecular and Optical Physics},
  year = {2012},
  volume = {45},
  number = {19},
  pages = {194013},
  url = {http://stacks.iop.org/0953-4075/45/i=19/a=194013}
}
Caillat J, Maquet A, Haessler S, Fabre B, Ruchon T, Salières P, Mairesse Y and Ta\ieb R (2011), "Attosecond Resolved Electron Release in Two-Color Near-Threshold Photoionization of N_2", Phys. Rev. Lett.., Mar, 2011. Vol. 106, pp. 093002. American Physical Society.
Abstract: We have simulated two-color photoionization of N2 by solving the time-dependent Schrödinger equation with a simple model accounting for the correlated vibronic dynamics of the molecule and of the ion N2+. Our results, in very good agreement with recent experiments [Haessler et al., Phys. Rev. A 80 011404 (2009)], show how a resonance embedded in the molecular continuum dramatically affects the phases of the two-photon transition amplitudes. In addition, we introduce a formal relation between these measurable phases and the photoelectron release time, opening the way to attosecond time-resolved measurements, equivalent to double-slit experiments in the time domain.
BibTeX:
@article{CaillatPRL2011,
  author = {Caillat, Jérémie and Maquet, Alfred and Haessler, Stefan and Fabre, Baptiste and Ruchon, Thierry and Salières, Pascal and Mairesse, Yann and Ta\ieb, Richard},
  title = {Attosecond Resolved Electron Release in Two-Color Near-Threshold Photoionization of N_2},
  journal = {Phys. Rev. Lett.},
  publisher = {American Physical Society},
  year = {2011},
  volume = {106},
  pages = {093002},
  url = {http://link.aps.org/doi/10.1103/PhysRevLett.106.093002},
  doi = {10.1103/PhysRevLett.106.093002}
}
Bourassin-Bouchet C, Diveki Z, de Rossi S, English E, Meltchakov E, Gobert O, Guénot D, Carré B, Delmotte F, Salières P and Ruchon T (2011), "Control of the attosecond synchronization of XUV radiation with phase-optimized mirrors", Opt. Express., Feb, 2011. Vol. 19(4), pp. 3809-3817. OSA.
Abstract: We report on the advanced amplitude and phase control of attosecond radiation allowed by specifically-designed multilayer XUV mirrors. We first demonstrate that such mirrors can compensate for the intrinsic chirp of the attosecond emission over a large bandwidth of more than 20 eV. We then show that their combination with metallic foils introduces a third-order dispersion that is adjustable through the mirror's incidence angle. This results in a controllable beating allowing the radiationto be shaped from a single to a series of sub-100 as pulses.
BibTeX:
@article{BourassinBouchetOE2011,
  author = {C. Bourassin-Bouchet and Z. Diveki and S. de Rossi and E. English and E. Meltchakov and O. Gobert and D. Guénot and B. Carré and F. Delmotte and P. Salières and T. Ruchon},
  title = {Control of the attosecond synchronization of XUV radiation with phase-optimized mirrors},
  journal = {Opt. Express},
  publisher = {OSA},
  year = {2011},
  volume = {19},
  number = {4},
  pages = {3809--3817},
  url = {http://www.opticsexpress.org/abstract.cfm?URI=oe-19-4-3809},
  doi = {10.1364/OE.19.003809}
}
Haessler S, Caillat J, Boutu W, Giovanetti-Teixeira C, Ruchon T, Auguste T, Diveki Z, Breger P, Maquet A, Carré B, Ta\ieb R and Salières P (2010), "Attosecond imaging of molecular electronic wavepackets", Nature Physics. Vol. 6(3), pp. 200-206.
BibTeX:
@article{HaesslerNP2010,
  author = {Haessler, S. and Caillat, J. and Boutu, W. and Giovanetti-Teixeira, C. and Ruchon, T. and Auguste, T. and Diveki, Z. and Breger, P. and Maquet, A. and Carré, B. and Ta\ieb, R. and Salières, P.},
  title = {Attosecond imaging of molecular electronic wavepackets},
  journal = {Nature Physics},
  year = {2010},
  volume = {6},
  number = {3},
  pages = {200-206},
  doi = {10.1038/NPHYS1511}
}
Swoboda M, Dahlström JM, Ruchon T, Johnsson P, Mauritsson J, L'Huillier A and Schafer KJ (2009), "Intensity dependence of laser-assisted attosecond photoionization spectra", Laser Physics., August, 2009. Vol. 19, pp. 1591-1599.
Abstract: We study experimentally the influence of the intensity of the infrared (IR) probe field on attosecond pulse train (APT) phase measurements performed with the RABITT method (Reconstruction of Attosecond Beating by Interference in Two-Photon Transitions). We find that if a strong IR field is applied, the attosecond pulses will appear to have lower-than-actual chirp rates. We also observe the onset of the streaking regime in the breakdown of the weak-field RABITT conditions. We perform a Fourier-analysis of harmonic and sideband continuum states and show that the mutual phase relation of the harmonics can be extracted from higher Fourier components.
BibTeX:
@article{SwobodaLP2009,
  author = {Swoboda, M. and Dahlström, J. M. and Ruchon, T. and Johnsson, P. and Mauritsson, J. and L'Huillier, A. and Schafer, K. J.},
  title = {Intensity dependence of laser-assisted attosecond photoionization spectra},
  journal = {Laser Physics},
  year = {2009},
  volume = {19},
  pages = {1591-1599},
  doi = {10.1134/S1054660X09150390}
}
Mansten E, Dahlström JM, Mauritsson J, Ruchon T, L'Huillier A, Tate J, Gaarde MB, Eckle P, Guandalini A, Holler M, Schapper F, Gallmann L and Keller U (2009), "Spectral Signature of Short Attosecond Pulse Trains", Phys. Rev. Lett.., Feb, 2009. Vol. 102(8), pp. 083002. American Physical Society.
Abstract: We report experimental measurements of high-order harmonic spectra generated in Ar using a carrier-envelope-offset (CEO) stabilized 12 fs, 800 nm laser field and a fraction (less than 10%) of its second harmonic. Additional spectral peaks are observed between the harmonic peaks, which are due to interferences between multiple pulses in the train. The position of these peaks varies with the CEO and their number is directly related to the number of pulses in the train. An analytical model, as well as numerical simulations, support our interpretation.
BibTeX:
@article{ManstenPRL2009,
  author = {Mansten, E. and Dahlström, J. M. and Mauritsson, J. and Ruchon, T. and L'Huillier, A. and Tate, J. and Gaarde, M. B. and Eckle, P. and Guandalini, A. and Holler, M. and Schapper, F. and Gallmann, L. and Keller, U.},
  title = {Spectral Signature of Short Attosecond Pulse Trains},
  journal = {Phys. Rev. Lett.},
  publisher = {American Physical Society},
  year = {2009},
  volume = {102},
  number = {8},
  pages = {083002},
  doi = {10.1103/PhysRevLett.102.083002}
}
He X, Miranda M, Schwenke J, Guilbaud O, Ruchon T, Heyl C, Georgadiou E, Rakowski R, Persson A, Gaarde MB and L'Huillier A (2009), "Spatial and spectral properties of the high-order harmonic emission in argon for seeding applications", Phys. Rev. A., Jun, 2009. Vol. 79(6), pp. 063829. American Physical Society.
Abstract: We characterize and control the harmonic emission in the spectral and spatial domains in order to define in which conditions the harmonic radiation can be a high-quality seed for soft x-ray and x-ray free-electron lasers. The length of the gas cell, where harmonics are generated, was optimized and the energy per pulse was determined in absolute value with a calibrated x-ray photodiode. The beam spatial profile was measured and, in some conditions, a very collimated beam with a half-angle divergence below 1 mrad could be obtained. We also show that increasing the intensity of the fundamental laser field leads to a considerable broadening of the bandwidth of the harmonic radiation, allowing us to cover a large spectral range. This effect is due to fundamental reshaping leading to an efficient phase matching of both short- and long-trajectory contributions.
BibTeX:
@article{HePRA2009,
  author = {He, Xinkui and Miranda, M. and Schwenke, J. and Guilbaud, O. and Ruchon, T. and Heyl, C. and Georgadiou, E. and Rakowski, R. and Persson, A. and Gaarde, M. B. and L'Huillier, A.},
  title = {Spatial and spectral properties of the high-order harmonic emission in argon for seeding applications},
  journal = {Phys. Rev. A},
  publisher = {American Physical Society},
  year = {2009},
  volume = {79},
  number = {6},
  pages = {063829},
  doi = {10.1103/PhysRevA.79.063829}
}
Haessler S, Fabre B, Higuet J, Caillat J, Ruchon T, Breger P, Carré B, Constant E, Maquet A, Mével E, Salières P, Ta\ieb R and Mairesse Y (2009), "Phase-resolved attosecond near-threshold photoionization of molecular nitrogen", Phys. Rev. A., Jul, 2009. Vol. 80(1), pp. 011404. American Physical Society.
Abstract: We photoionize nitrogen molecules with a train of extreme ultraviolet attosecond pulses together with a weak infrared field. We measure the phase of the two-color two-photon ionization transition (molecular phase) for different states of the ion. We observe a 0.9pi shift for the electrons produced in the ionization channels leading to the Xâ??2Σg+, vâ?²=1, and vâ?²=2 states. We relate this phase shift to the presence of a complex resonance in the continuum. By providing both a high spectral and temporal resolution, this general approach gives access to the evolution of extremely short-lived states, which is often not accessible otherwise.
BibTeX:
@article{HaesslerPRA2009,
  author = {Haessler, S. and Fabre, B. and Higuet, J. and Caillat, J. and Ruchon, T. and Breger, P. and Carré, B. and Constant, E. and Maquet, A. and Mével, E. and Salières, P. and Ta\ieb, R. and Mairesse, Y.},
  title = {Phase-resolved attosecond near-threshold photoionization of molecular nitrogen},
  journal = {Phys. Rev. A},
  publisher = {American Physical Society},
  year = {2009},
  volume = {80},
  number = {1},
  pages = {011404},
  doi = {10.1103/PhysRevA.80.011404}
}
Dahlström JM, Fordell T, Mansten E, Ruchon T, Swoboda M, Klünder K, Gisselbrecht M, L'Huillier A and Mauritsson J (2009), "Atomic and macroscopic measurements of attosecond pulse trains", Phys. Rev. A., Sep, 2009. Vol. 80(3), pp. 033836. American Physical Society.
Abstract: We characterize attosecond pulses in a train using both the well established â??reconstruction of attosecond beating by interference of two-photon transitionsâ?? (RABITT) technique and the recently demonstrated in situ method, which is based on a weak perturbation of the harmonic generation process by the second harmonic of the laser field. The latter technique determines the characteristics of the single atom emission, while RABITT allows one to measure attosecond pulses â??on target.â?? By comparing the results of the two methods, the influence of propagation and filtering on the attosecond pulses can be extracted.
BibTeX:
@article{DahlstromPRA2009,
  author = {Dahlström, J. M. and Fordell, T. and Mansten, E. and Ruchon, T. and Swoboda, M. and Klünder, K. and Gisselbrecht, M. and L'Huillier, A. and Mauritsson, J.},
  title = {Atomic and macroscopic measurements of attosecond pulse trains},
  journal = {Phys. Rev. A},
  publisher = {American Physical Society},
  year = {2009},
  volume = {80},
  number = {3},
  pages = {033836},
  doi = {10.1103/PhysRevA.80.033836}
}
Ruchon T, Hauri CP, Varjú K, Mansten E, Swoboda M, López-Martens R and L'Huillier A (2008), "Macroscopic effects in attosecond pulse generation", New Journal of Physics. Vol. 10(2), pp. 025027 (10pp).
Abstract: We examine how the generation and propagation of high-order harmonics in a partly ionized gas medium affect their strength and synchronization. The temporal properties of the resulting attosecond pulses generated in long gas targets can be significantly influenced by macroscopic effects, in particular by the intensity in the medium and the degree of ionization which control the dispersion. Under some conditions, the use of gas targets longer than the absorption length can lead to the generation of compressed attosecond pulses. We show these macroscopic effects experimentally, using a 6 mm-long argon-filled gas cell as the generating medium.
BibTeX:
@article{RuchonNJP2008,
  author = {T Ruchon and C P Hauri and K Varjú and E Mansten and M Swoboda and R López-Martens and A L'Huillier},
  title = {Macroscopic effects in attosecond pulse generation},
  journal = {New Journal of Physics},
  year = {2008},
  volume = {10},
  number = {2},
  pages = {025027 (10pp)},
  url = {http://stacks.iop.org/1367-2630/10/025027}
}
Mauritsson J, Johnsson P, Mansten E, Swoboda M, Ruchon T, L'Huillier A and Schafer KJ (2008), "Coherent Electron Scattering Captured by an Attosecond Quantum Stroboscope", Phys. Rev. Lett.. Vol. 100(7), pp. 073003. APS.
Abstract: We demonstrate a quantum stroboscope based on a sequence of identical attosecond pulses that are used to release electrons into a strong infrared (IR) laser field exactly once per laser cycle. The resulting electron momentum distributions are recorded as a function of time delay between the IR laser and the attosecond pulse train using a velocity map imaging spectrometer. Because our train of attosecond pulses creates a train of identical electron wave packets, a single ionization event can be studied stroboscopically. This technique has enabled us to image the coherent electron scattering that takes place when the IR field is sufficiently strong to reverse the initial direction of the electron motion causing it to rescatter from its parent ion.
BibTeX:
@article{MauritssonPRL2008,
  author = {J. Mauritsson and P. Johnsson and E. Mansten and M. Swoboda and T. Ruchon and A. L'Huillier and K. J. Schafer},
  title = {Coherent Electron Scattering Captured by an Attosecond Quantum Stroboscope},
  journal = {Phys. Rev. Lett.},
  publisher = {APS},
  year = {2008},
  volume = {100},
  number = {7},
  pages = {073003},
  url = {http://link.aps.org/abstract/PRL/v100/e073003},
  doi = {10.1103/PhysRevLett.100.073003}
}
Gustafsson E, Ruchon T, Swoboda M, Remetter T, Pourtal E, López-Martens R, Balcou P and L'Huillier A (2007), "Broadband attosecond pulse shaping", Opt. Lett.. Vol. 32(11), pp. 1353-1355. OSA.
Abstract: We use semiconductor (Si) and metallic (Al, Zr) transmission filters to shape, in amplitude and phase, high-order harmonics generated from the interaction of an intense titanium sapphire laser field with a pulsed neon gas target. Depending on the properties of the filter, the emitted attosecond pulses can be optimized in bandwidth and/or pulse length. We demonstrate the generation of attosecond pulses centered at energies from 50 to 80 eV, with bandwidths as large as 45 eV and with pulse durations compressed to 130 as.
BibTeX:
@article{GustafssonOL2007,
  author = {E. Gustafsson and T. Ruchon and M. Swoboda and T. Remetter and E. Pourtal and R. López-Martens and Ph. Balcou and A. L'Huillier},
  title = {Broadband attosecond pulse shaping},
  journal = {Opt. Lett.},
  publisher = {OSA},
  year = {2007},
  volume = {32},
  number = {11},
  pages = {1353--1355},
  url = {http://ol.osa.org/abstract.cfm?URI=ol-32-11-1353}
}
Varjú K, Johnsson P, Mauritsson J, Remetter T, Ruchon T, Ni Y, Lépine F, Kling M, Khan J, Schafer KJ, Vrakking MJJ and L'Huillier A (2006), "Angularly resolved electron wave packet interferences", Journal of Physics B: Atomic, Molecular and Optical Physics. Vol. 39(18), pp. 3983-3991.
Abstract: We study experimentally the ionization of argon atoms by a train of attosecond pulses in the presence of a strong infrared laser field, using a velocity map imaging technique. The recorded momentum distribution strongly depends on the delay between the attosecond pulses and the laser field. We interpret the interference patterns observed for different delays using numerical and analytical calculations within the strong field approximation.
BibTeX:
@article{VarjuJPB2006,
  author = {K Varjú and P Johnsson and J Mauritsson and T Remetter and T Ruchon and Y Ni and F Lépine and M Kling and J Khan and K J Schafer and M J J Vrakking and A L'Huillier},
  title = {Angularly resolved electron wave packet interferences},
  journal = {Journal of Physics B: Atomic, Molecular and Optical Physics},
  year = {2006},
  volume = {39},
  number = {18},
  pages = {3983-3991},
  url = {http://stacks.iop.org/0953-4075/39/3983}
}
Ruchon T, Vallet M, Chauvat D and Le Floch A (2006), "A dipole interaction model for magnetochiral birefringence", The Journal of Chemical Physics., August, 2006. Vol. 125, pp. 4104-+.
BibTeX:
@article{ruchonjcp2006,
  author = {Ruchon, T. and Vallet, M. and Chauvat, D. and Le Floch, A.},
  title = {A dipole interaction model for magnetochiral birefringence},
  journal = {The Journal of Chemical Physics},
  year = {2006},
  volume = {125},
  pages = {4104-+},
  doi = {10.1063/1.2211613}
}
Ruchon T, Thepot J-Y, Vallet M and Floch AL (2006), "Magneto-optical properties of diastereoisomers", Journal de physique IV. Vol. 135, pp. 271-272.
BibTeX:
@article{ruchon2006JP,
  author = {T. Ruchon and J.-Y. Thepot and M. Vallet and A. Le Floch},
  title = {Magneto-optical properties of diastereoisomers},
  journal = {Journal de physique IV},
  year = {2006},
  volume = {135},
  pages = {271-272}
}
Ruchon T, Vallet M, Chauvat D, Floch AL and Thépot J-Y (2005), "Experimental investigation of the magnetochiral index in liquids", Phys. Rev. A. Vol. 72, pp. 043405.
BibTeX:
@article{ruchon2005,
  author = {T. Ruchon and M. Vallet and D. Chauvat and A. Le Floch and and J.-Y. Thépot},
  title = {Experimental investigation of the magnetochiral index in liquids},
  journal = {Phys. Rev. A},
  year = {2005},
  volume = {72},
  pages = {043405}
}
Ruchon T, Thépot J-Y, Vallet M and Floch AL (2005), "The magneto-optical properties of diastereoisomers", Chem. Phys. Lett.. Vol. 412, pp. 411-415.
BibTeX:
@article{ruchon2005CPL,
  author = {T. Ruchon and J.-Y. Thépot and M. Vallet and A. Le Floch},
  title = {The magneto-optical properties of diastereoisomers},
  journal = {Chem. Phys. Lett.},
  year = {2005},
  volume = {412},
  pages = {411-415}
}
Ruchon T, Vallet M, Thépot J-Y, Floch AL and Boyd RW (2004), "Experimental evidence of magnetochiral interaction in Pasteur's tartrates", C.R.A.S. : Physique. Vol. 5, pp. 273-277.
BibTeX:
@article{ruchon2004,
  author = {T. Ruchon and M. Vallet and J.-Y. Thépot and A. Le Floch and R. W. Boyd},
  title = {Experimental evidence of magnetochiral interaction in Pasteur's tartrates},
  journal = {C.R.A.S. : Physique},
  year = {2004},
  volume = {5},
  pages = {273-277}
}
Ruchon T, Thepot J-Y, Vallet M and Floch AL (2004), "Interpretation of magnetochiral birefringence using a dipole-dipole interaction model", Journal de physique IV. Vol. 119, pp. 265-266.
BibTeX:
@article{ruchon2004JP,
  author = {T. Ruchon and J.-Y. Thepot and M. Vallet and A. Le Floch},
  title = {Interpretation of magnetochiral birefringence using a dipole-dipole interaction model},
  journal = {Journal de physique IV},
  year = {2004},
  volume = {119},
  pages = {265-266}
}
Bonnet C, Bretenaker F, Brunel M, Chauvat D, Emile O, Lai N, Floch AL, Ropars G, Ruchon T, Singh K, Thepot J-Y and Vallet M (2002), "Magnetochirality and stochastic resonance in lasers", Journal de physique IV. Vol. 12, pp. PR5.
BibTeX:
@article{bonnet2004JP,
  author = {C. Bonnet and F. Bretenaker and M. Brunel and D. Chauvat and O. Emile and N.D. Lai and A. Le Floch and G. Ropars and T. Ruchon and K. Singh and J.-Y. Thepot and M. Vallet},
  title = {Magnetochirality and stochastic resonance in lasers},
  journal = {Journal de physique IV},
  year = {2002},
  volume = {12},
  pages = {PR5}
}
Vallet M, Ghosh R, Floch AL, Ruchon T, Bretenaker F and Thépot J-Y (2001), "Observation of Magnetochiral Birefringence", Phys. Rev. Lett.. Vol. 87, pp. 1830031-1830034.
BibTeX:
@article{vallet2001,
  author = {M. Vallet and R. Ghosh and A. Le Floch and T. Ruchon and F. Bretenaker and J.-Y. Thépot},
  title = {Observation of Magnetochiral Birefringence},
  journal = {Phys. Rev. Lett.},
  year = {2001},
  volume = {87},
  pages = {1830031-1830034}
}
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